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  • Defect Graphene as a Trifunctional Catalyst for Electrochemical Reactions

    Author(s)
    Jia, Yi
    Zhang, Longzhou
    Du, Aijun
    Gao, Guoping
    Chen, Jun
    Yan, Xuecheng
    Brown, Christopher L
    Yao, Xiangdong
    Griffith University Author(s)
    Yan, Xuecheng
    Jia, Yi
    Year published
    2016
    Metadata
    Show full item record
    Abstract
    Defects derived by the removal of heteroatoms from graphene are demonstrated, both experimentally and theoretically, to be effective for all three basic electrochemical reactions, e.g., oxygen reduction (ORR), oxygen evolution (OER), and hydrogen evolution (HER). Density function theory calculations further reveal that the different types of defects are essential for the individual electrocatalytic activity for ORR, OER, and HER, respectively.Defects derived by the removal of heteroatoms from graphene are demonstrated, both experimentally and theoretically, to be effective for all three basic electrochemical reactions, e.g., oxygen reduction (ORR), oxygen evolution (OER), and hydrogen evolution (HER). Density function theory calculations further reveal that the different types of defects are essential for the individual electrocatalytic activity for ORR, OER, and HER, respectively.
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    Journal Title
    Advanced Materials
    Volume
    28
    Issue
    43
    DOI
    https://doi.org/10.1002/adma.201602912
    Subject
    Physical sciences
    Chemical sciences
    Physical properties of materials
    Engineering
    Publication URI
    http://hdl.handle.net/10072/100203
    Collection
    • Journal articles

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