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  • Iron-Based Metal-Organic Frameworks as Catalysts for Visible Light-Driven Water Oxidation

    Author(s)
    Chi, Le
    Xu, Qian
    Liang, Xiaoyu
    Wang, Jide
    Su, Xintai
    Griffith University Author(s)
    Su, Xintai
    Year published
    2016
    Metadata
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    Abstract
    The development of earth-abundant, active, and stable catalysts is important for solar energy conversion. Metal-organic frameworks (MOFs) have been viewed as a promising class of porous materials, which may have innovative application in photocatalysis. In this paper, three types of Fe-based MOFs and their aminofunctionalized derivatives have been fabricated and systematically studied as water oxidation catalysts (WOCs) for oxygen evolution under visible light irradiation. MIL-101(Fe) possesses a higher current density and earlier onset potential and exhibits excellent visible light-driven oxygen evolution activity than the ...
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    The development of earth-abundant, active, and stable catalysts is important for solar energy conversion. Metal-organic frameworks (MOFs) have been viewed as a promising class of porous materials, which may have innovative application in photocatalysis. In this paper, three types of Fe-based MOFs and their aminofunctionalized derivatives have been fabricated and systematically studied as water oxidation catalysts (WOCs) for oxygen evolution under visible light irradiation. MIL-101(Fe) possesses a higher current density and earlier onset potential and exhibits excellent visible light-driven oxygen evolution activity than the other Fe-based catalysts. It speeds up the oxygen evolution reaction rate with the higher initial turnover frequencies value of 0.10 s−1. Our study demonstrates that Fe-based MOFs as efficient WOCs are promising candidates for photocatalytic water oxidation process.
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    Journal Title
    Small
    Volume
    12
    Issue
    10
    DOI
    https://doi.org/10.1002/smll.201503526
    Subject
    Physical Chemistry not elsewhere classified
    Publication URI
    http://hdl.handle.net/10072/172077
    Collection
    • Journal articles

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