Efficient Excitation of Multiple Plasmonic Modes on Three-Dimensional Graphene: An Unexplored Dimension
Author(s)
Song, Jingchao
Zhang, Lei
Xue, Yunzhou
Wu, Qing Yang Steve
Xia, Fang
Zhang, Chao
Zhong, Yu-Lin
Zhang, Yupeng
Teng, Jinghua
Premaratne, Malin
Qiu, Cheng-Wei
Bao, Qiaoliang
Griffith University Author(s)
Year published
2016
Metadata
Show full item recordAbstract
Graphene is a typical two-dimensional (2D) allotrope form of carbon. Excellent optical and electric properties of graphene, such as broadband absorption and high mobility of carriers, promise prosperous applications in optic and optoelectronic devices. However, flat graphene structures (either graphene film on a structural substrate or structural graphene) hardly support efficient excitation of high-order plasmonic modes, which results in a serious deficiency in realizing efficient light–matter interaction in graphene-based devices. Here, by configuring the flat graphene into complex three-dimensional (3D) pillars, strong ...
View more >Graphene is a typical two-dimensional (2D) allotrope form of carbon. Excellent optical and electric properties of graphene, such as broadband absorption and high mobility of carriers, promise prosperous applications in optic and optoelectronic devices. However, flat graphene structures (either graphene film on a structural substrate or structural graphene) hardly support efficient excitation of high-order plasmonic modes, which results in a serious deficiency in realizing efficient light–matter interaction in graphene-based devices. Here, by configuring the flat graphene into complex three-dimensional (3D) pillars, strong high-order plasmonic modes were observed and verified numerically and experimentally. It is found that, despite the influence of geometry and material parameters on resonance, the excitation efficiency of high-order modes is highly dependent on the graphene on the sidewall of pillars. Therefore, the proposed 3D graphene structures not only retain the merits of 2D materials but also introduce a new dimension to control the light–matter interaction. In addition, the fabrication technique in this work can be readily applied to other 2D materials with various geometric shapes. It is believed that the proposed 3D form of 2D materials will ignite a plethora of unprecedented designs and applications in THz communication such as THz pulse generators, modulators, detectors, and spectrometers.
View less >
View more >Graphene is a typical two-dimensional (2D) allotrope form of carbon. Excellent optical and electric properties of graphene, such as broadband absorption and high mobility of carriers, promise prosperous applications in optic and optoelectronic devices. However, flat graphene structures (either graphene film on a structural substrate or structural graphene) hardly support efficient excitation of high-order plasmonic modes, which results in a serious deficiency in realizing efficient light–matter interaction in graphene-based devices. Here, by configuring the flat graphene into complex three-dimensional (3D) pillars, strong high-order plasmonic modes were observed and verified numerically and experimentally. It is found that, despite the influence of geometry and material parameters on resonance, the excitation efficiency of high-order modes is highly dependent on the graphene on the sidewall of pillars. Therefore, the proposed 3D graphene structures not only retain the merits of 2D materials but also introduce a new dimension to control the light–matter interaction. In addition, the fabrication technique in this work can be readily applied to other 2D materials with various geometric shapes. It is believed that the proposed 3D form of 2D materials will ignite a plethora of unprecedented designs and applications in THz communication such as THz pulse generators, modulators, detectors, and spectrometers.
View less >
Journal Title
ACS Photonics
Volume
3
Issue
10
Subject
Atomic, molecular and optical physics
Quantum physics
Functional materials