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dc.contributor.authorEvans, Denis J.
dc.contributor.authorBernhardt, Debra
dc.contributor.authorWilliams, Stephen R.
dc.contributor.editorDonald Levy
dc.date.accessioned2017-05-03T12:18:45Z
dc.date.available2017-05-03T12:18:45Z
dc.date.issued2008
dc.date.modified2009-04-02T07:16:05Z
dc.identifier.issn0021-9606
dc.identifier.doi10.1063/1.2812241
dc.identifier.urihttp://hdl.handle.net/10072/21822
dc.description.abstractRecently, there has been considerable interest in the fluctuation theorem (FT). The Evans-Searles FT shows how time reversible microscopic dynamics leads to irreversible macroscopic behavior as the system size or observation time increases. We show that the argument of this FT, the dissipation function, plays a central role in nonlinear response theory and derive the dissipation theorem, giving exact relations for nonlinear response of classical N-body systems that are more widely applicable than previous expressions. These expressions should be verifiable experimentally. When linearized they reduce to the well-known Green-Kubo expressions for linear response.
dc.description.peerreviewedYes
dc.description.publicationstatusYes
dc.format.extent437320 bytes
dc.format.mimetypeapplication/pdf
dc.languageEnglish
dc.language.isoeng
dc.publisherAmerican Institute of Physics
dc.publisher.placeUnited States
dc.publisher.urihttp://jcp.aip.org/
dc.relation.ispartofstudentpublicationN
dc.relation.ispartofpagefrom014504.1
dc.relation.ispartofpageto014504.6
dc.relation.ispartofjournalJournal of Chemical Physics
dc.relation.ispartofvolume128
dc.rights.retentionY
dc.subject.fieldofresearchPhysical sciences
dc.subject.fieldofresearchChemical sciences
dc.subject.fieldofresearchEngineering
dc.subject.fieldofresearchcode51
dc.subject.fieldofresearchcode34
dc.subject.fieldofresearchcode40
dc.titleOn the fluctuation theorem for the dissipation function and its connection with response theory.
dc.typeJournal article
dc.type.descriptionC1 - Articles
dc.type.codeC - Journal Articles
gro.rights.copyright© 2008 American Institute of Physics. This article may be downloaded for personal use only. Any other use requires prior permission of the author and the American Institute of Physics. along with the following message: The following article appeared in J. Chem. Phys. 128, 014504 (2008) and may be found at http://dx.doi.org/10.1063/1.2812241
gro.date.issued2008
gro.hasfulltextFull Text
gro.griffith.authorBernhardt, Debra J.


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