Characterization of aerosol over the Northern South China Sea during two cruises in 2003
Author(s)
Zhang, Xingying
Zhuang, Guoshun
Guo, Jinghua
Yin, Kedong
Zhang, Peng
Griffith University Author(s)
Year published
2007
Metadata
Show full item recordAbstract
Atmospheric transport of trace elements has been found to be an important pathway for their input to the ocean. TSP, PM10, and PM2.5 aerosol samples were collected over the Northern South China Sea in two cruises in 2003 to estimate the input of aerosol from continent to the ocean. About 23 elements and 14 soluble ions in aerosol samples were measured. The average mass concentration of TSP in Cruise I in January (78 姭-3) was ~twice of that in Cruise II in April (37 姭-3). Together with the crustal component, heavy metals from pollution sources over the land (especially from the industry and automobiles in Guangzhou) were ...
View more >Atmospheric transport of trace elements has been found to be an important pathway for their input to the ocean. TSP, PM10, and PM2.5 aerosol samples were collected over the Northern South China Sea in two cruises in 2003 to estimate the input of aerosol from continent to the ocean. About 23 elements and 14 soluble ions in aerosol samples were measured. The average mass concentration of TSP in Cruise I in January (78 姭-3) was ~twice of that in Cruise II in April (37 姭-3). Together with the crustal component, heavy metals from pollution sources over the land (especially from the industry and automobiles in Guangzhou) were transported to and deposited into the ocean. The atmospheric MSA concentrations in PM2.5 (0.048 姭-3 in Cruise I and 0.043 姭-3 in Cruise II) over Northern South China Sea were comparable to those over other coastal regions. The ratio of non-sea-salt (NSS)-sulfate to MSA is 103-655 for Cruise I and 15-440 for Cruise II in PM2.5 samples, which were much higher than those over remote oceans. The estimated anthropogenic sulfate accounts for 83-98% in Cruise I and 63-95% in Cruise II of the total NSS-sulfate. Fe (II) concentration in the aerosols collected over the ocean ranged from 0.1 to 0.9 mgm 3, accounting for 16-82% of the total iron in the aerosol, which could affect the marine biogeochemical cycle greatly.
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View more >Atmospheric transport of trace elements has been found to be an important pathway for their input to the ocean. TSP, PM10, and PM2.5 aerosol samples were collected over the Northern South China Sea in two cruises in 2003 to estimate the input of aerosol from continent to the ocean. About 23 elements and 14 soluble ions in aerosol samples were measured. The average mass concentration of TSP in Cruise I in January (78 姭-3) was ~twice of that in Cruise II in April (37 姭-3). Together with the crustal component, heavy metals from pollution sources over the land (especially from the industry and automobiles in Guangzhou) were transported to and deposited into the ocean. The atmospheric MSA concentrations in PM2.5 (0.048 姭-3 in Cruise I and 0.043 姭-3 in Cruise II) over Northern South China Sea were comparable to those over other coastal regions. The ratio of non-sea-salt (NSS)-sulfate to MSA is 103-655 for Cruise I and 15-440 for Cruise II in PM2.5 samples, which were much higher than those over remote oceans. The estimated anthropogenic sulfate accounts for 83-98% in Cruise I and 63-95% in Cruise II of the total NSS-sulfate. Fe (II) concentration in the aerosols collected over the ocean ranged from 0.1 to 0.9 mgm 3, accounting for 16-82% of the total iron in the aerosol, which could affect the marine biogeochemical cycle greatly.
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Journal Title
Atmospheric Environment
Volume
41
Publisher URI
Subject
Atmospheric Sciences not elsewhere classified
Statistics
Atmospheric Sciences
Environmental Engineering