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  • Strategies for Improving the Functionality of Zeolitic Imidazolate Frameworks: Tailoring Nanoarchitectures for Functional Applications

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    KanetiPUB2208.pdf (3.878Mb)
    Author(s)
    Kaneti, Yusuf Valentino
    Dutta, Saikat
    Hossain, Md SA
    Shiddiky, Muhammad JA
    Tung, Kuo-Lun
    Shieh, Fa-Kuen
    Tsung, Chia-Kuang
    Wu, Kevin C-W
    Yamauchi, Yusuke
    Griffith University Author(s)
    Shiddiky, Muhammad J.
    Year published
    2017
    Metadata
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    Abstract
    Zeolitic imidazolate frameworks (ZIFs), a subclass of metal–organic frameworks (MOFs) built with tetrahedral metal ions and imidazolates, offer permanent porosity and high thermal and chemical stabilities. While ZIFs possess some attractive physical and chemical properties, it remains important to enhance their functionality for practical application. Here, an overview of the extensive strategies which have been developed to improve the functionality of ZIFs is provided, including linker modifications, functional hybridization of ZIFs via the encapsulation of guest species (such as metal and metal oxide nanoparticles and ...
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    Zeolitic imidazolate frameworks (ZIFs), a subclass of metal–organic frameworks (MOFs) built with tetrahedral metal ions and imidazolates, offer permanent porosity and high thermal and chemical stabilities. While ZIFs possess some attractive physical and chemical properties, it remains important to enhance their functionality for practical application. Here, an overview of the extensive strategies which have been developed to improve the functionality of ZIFs is provided, including linker modifications, functional hybridization of ZIFs via the encapsulation of guest species (such as metal and metal oxide nanoparticles and biomolecules) into ZIFs, and hybridization with polymeric matrices to form mixed matrix membranes for industrial gas and liquid separations. Furthermore, the developed strategies for achieving size and shape control of ZIF nanocrystals are considered, which are important for optimizing the textural characteristics as well as the functional performance of ZIFs and their derived materials/hybrids. Moreover, the recent trends of using ZIFs as templates for the derivation of nanoporous hybrid materials, including carbon/metal, carbon/oxide, carbon/sulfide, and carbon/phosphide hybrids, are discussed. Finally, some perspectives on the potential future research directions and applications for ZIFs and ZIF-derived materials are offered.
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    Journal Title
    Advanced Materials
    DOI
    https://doi.org/10.1002/adma.201700213
    Copyright Statement
    © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. This is the peer reviewed version of the following article: Strategies for Improving the Functionality of Zeolitic Imidazolate Frameworks: Tailoring Nanoarchitectures for Functional Applications, Advanced Materials, 2017 which has been published in final form at 10.1002/adma.201700213. This article may be used for non-commercial purposes in accordance with Wiley Terms and Conditions for Self-Archiving (http://olabout.wiley.com/WileyCDA/Section/id-820227.html#terms)
    Note
    This publication has been entered into Griffith Research Online as an Advanced Online Version.
    Subject
    Nanotechnology not elsewhere classified
    Physical Sciences
    Chemical Sciences
    Engineering
    Publication URI
    http://hdl.handle.net/10072/344967
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    • Journal articles

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