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dc.contributor.authorCao, Aihui
dc.contributor.authorZhang, Lijuan
dc.contributor.authorWang, Yun
dc.contributor.authorZhao, Huijun
dc.contributor.authorDeng, Hong
dc.contributor.authorLiu, Xueming
dc.contributor.authorLin, Zhang
dc.contributor.authorSu, Xintai
dc.contributor.authorYue, Fan
dc.date.accessioned2019-08-27T04:14:20Z
dc.date.available2019-08-27T04:14:20Z
dc.date.issued2019
dc.identifier.issn2168-0485
dc.identifier.doi10.1021/acssuschemeng.8b05396
dc.identifier.urihttp://hdl.handle.net/10072/386727
dc.description.abstractOn the basis of ultrathin two-dimensional (2D) nickel metal organic framework (UNiMOF) nanoflakes and 2D g-C3N4 nanoflakes, fresh visible-light-driven 2D/2D heterostructure catalysts were designed, which were assembled with a simplistic electrostatic self-assembly process. The photocatalytic performance of UNiMOF/g-C3N4 for H2 production was evaluated in visible light. The hydrogen evolution of 25.0% UNiMOF/g-C3N4 (UNG-25.0) heterojunction was 20.03 μmol h–1, which was greater than that of pure g-C3N4. In addition, the UNG composites also presented more excellent photocatalytic activity than that of bulk NiMOF/g-C3N4 (BNG) hybrid. This enhanced performance may depend on cooperative potentiation between UNiMOF and g-C3N4 efficiently lowering recombination of carriers. This work showed that constructing 2D–2D heterojunctions provides a feasible approach to obtain highly capable catalysts for photocatalytic decomposition of water.
dc.description.peerreviewedYes
dc.languageEnglish
dc.language.isoeng
dc.publisherAmerican Chemical Society
dc.relation.ispartofpagefrom2492
dc.relation.ispartofpageto2499
dc.relation.ispartofissue2
dc.relation.ispartofjournalACS Sustainable Chemistry and Engineering
dc.relation.ispartofvolume7
dc.subject.fieldofresearchAnalytical Chemistry
dc.subject.fieldofresearchEnvironmental Science and Management
dc.subject.fieldofresearchChemical Engineering
dc.subject.fieldofresearchcode0301
dc.subject.fieldofresearchcode0502
dc.subject.fieldofresearchcode0904
dc.subject.keywordsScience & Technology
dc.subject.keywordsPhysical Sciences
dc.subject.keywordsTechnology
dc.subject.keywordsChemistry, Multidisciplinary
dc.subject.keywordsGreen & Sustainable Science & Technology
dc.title2D-2D Heterostructured UNiMOF/g-C3N4 for Enhanced Photocatalytic H-2 Production under Visible-Light Irradiation
dc.typeJournal article
dc.type.descriptionC1 - Articles
dcterms.bibliographicCitationCao, A; Zhang, L; Wang, Y; Zhao, H; Deng, H; Liu, X; Lin, Z; Su, X; Yue, F, 2D-2D Heterostructured UNiMOF/g-C3N4 for Enhanced Photocatalytic H-2 Production under Visible-Light Irradiation, ACS Sustainable Chemistry and Engineering, 2019, 7 (2), pp. 2492-2499
dc.date.updated2019-08-27T04:10:46Z
gro.hasfulltextNo Full Text
gro.griffith.authorWang, Yun
gro.griffith.authorZhao, Huijun


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