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dc.contributor.authorZhang, Le
dc.contributor.authorMao, Fangxin
dc.contributor.authorZheng, Li Rong
dc.contributor.authorWang, Hai Feng
dc.contributor.authorYang, Xiao Hua
dc.contributor.authorYang, Hua Gui
dc.date.accessioned2019-09-25T03:32:16Z
dc.date.available2019-09-25T03:32:16Z
dc.date.issued2018
dc.identifier.issn2155-5435
dc.identifier.doi10.1021/acscatal.8b03789
dc.identifier.urihttp://hdl.handle.net/10072/387728
dc.description.abstractElectrochemical CO2 reduction reaction (CO2RR) has attracted significant interest in the storage of renewable solar energy and mitigation of environmental issues. Here, we report a strategy to tune metal electrocatalyst by means of metal-substrate interactions to boost CO2RR process. It was found that carbon nitride (C3N4) supported Au nanoparticles (Au/C3N4) exhibit a better performance than carbon-supported Au nanoparticles (Au/C). The combined experimental and theoretical results evidence that Au-C3N4 interaction induces the formation of negatively charged Au surface, which could stabilize the key intermediateCOOH. Similar enhanced CO2RR performance is also observed on C3N4 supported Ag nanoparticles (Ag/C3N4), demonstrating the universality of this strategy for enhancing CO2RR.
dc.description.peerreviewedYes
dc.languageEnglish
dc.language.isoeng
dc.publisherAmerican Chemical Society (ACS Publications)
dc.relation.ispartofpagefrom11035
dc.relation.ispartofpageto11041
dc.relation.ispartofissue12
dc.relation.ispartofjournalACS Catalysis
dc.relation.ispartofvolume8
dc.subject.fieldofresearchInorganic Chemistry
dc.subject.fieldofresearchOrganic Chemistry
dc.subject.fieldofresearchChemical Engineering
dc.subject.fieldofresearchcode0302
dc.subject.fieldofresearchcode0305
dc.subject.fieldofresearchcode0904
dc.subject.keywordsScience & Technology
dc.subject.keywordsPhysical Sciences
dc.subject.keywordsChemistry, Physical
dc.subject.keywordsCO2 electroreduction
dc.titleTuning Metal Catalyst with Metal-C3N4 Interaction for Efficient CO2 Electroreduction
dc.typeJournal article
dc.type.descriptionC1 - Articles
dcterms.bibliographicCitationZhang, L; Mao, F; Zheng, LR; Wang, HF; Yang, XH; Yang, HG, Tuning Metal Catalyst with Metal-C3N4 Interaction for Efficient CO2 Electroreduction, ACS CATALYSIS, 2018, 8 (12), pp. 11035-11041
dc.date.updated2019-09-25T03:30:28Z
gro.hasfulltextNo Full Text
gro.griffith.authorYang, Huagui


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