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dc.contributor.authorLi, Xiaomin
dc.contributor.authorGuo, Zhenzhen
dc.contributor.authorZhao, Tiancong
dc.contributor.authorLu, Yang
dc.contributor.authorZhou, Lei
dc.contributor.authorZhao, Dongyuan
dc.contributor.authorZhang, Fan
dc.date.accessioned2019-10-04T06:47:52Z
dc.date.available2019-10-04T06:47:52Z
dc.date.issued2016
dc.identifier.issn1433-7851
dc.identifier.doi10.1002/anie.201510609
dc.identifier.urihttp://hdl.handle.net/10072/388105
dc.description.abstractLanthanide doped core-multishell structured NaGdF4:Yb,Er@NaYF4:Yb@NaGdF4:Yb,Nd@NaYF4@NaGdF4:Yb,Tm@NaYF4 nanoparticles with power-density independent orthogonal excitations-emissions upconversion luminescence (UCL) were fabricated for the first time. The optical properties of these core-multishell structured nanoparticles were related to the absorption filtration effect of the NaGdF4:Yb,Tm layer. By tuning the thickness of the filtration layer, the nanoparticles can exhibit unique two independent groups of UCL: Tm3+ prominent UV/blue (UV=ultraviolet) UCL under the excitation at 980nm and Er3+ prominent green/red UCL under the excitation at 796nm. The filtration-shell mediated orthogonal excitations-emissions UCL are power-density independent. As a proof of concept, the core-multishell nanoparticles are used in multi-dimensional security design and imaging-guided combined photodynamic therapy and chemotherapy. A different light: Lanthanide-doped nanoparticles (NPs) with a filtration shell that separates two different luminescence processes and prevents them from interfering with each other are prepared. The filtration effects allow the core-multishell upconversion NPs to show power density independent orthogonal excitations-emissions luminescence and be used in anti-counterfeiting and imaging-guided combined therapy.
dc.description.peerreviewedYes
dc.languageEnglish
dc.language.isoeng
dc.publisherWiley Blackwell
dc.relation.ispartofpagefrom2464
dc.relation.ispartofpageto2469
dc.relation.ispartofissue7
dc.relation.ispartofjournalAngewandte Chemie, International Edition
dc.relation.ispartofvolume55
dc.subject.fieldofresearchChemical Sciences
dc.subject.fieldofresearchcode03
dc.subject.keywordsScience & Technology
dc.subject.keywordsPhysical Sciences
dc.subject.keywordsChemistry, Multidisciplinary
dc.subject.keywordsanti-counterfeiting
dc.titleFiltration Shell Mediated Power Density Independent Orthogonal Excitations-Emissions Upconversion Luminescence
dc.typeJournal article
dc.type.descriptionC1 - Articles
dcterms.bibliographicCitationLi, X; Guo, Z; Zhao, T; Lu, Y; Zhou, L; Zhao, D; Zhang, F, Filtration Shell Mediated Power Density Independent Orthogonal Excitations-Emissions Upconversion Luminescence, Angewandte Chemie, International Edition, 2016, 55 (7), pp. 2464-2469
dc.date.updated2019-10-04T06:46:28Z
gro.hasfulltextNo Full Text
gro.griffith.authorZhao, Dongyuan


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