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dc.contributor.authorBatmunkh, Munkhbayar
dc.contributor.authorShrestha, Aabhash
dc.contributor.authorBat-Erdene, Munkhjargal
dc.contributor.authorNine, Md Julker
dc.contributor.authorShearer, Cameron J
dc.contributor.authorGibson, Christopher T
dc.contributor.authorSlattery, Ashley D
dc.contributor.authorTawfik, Sherif Abdulkader
dc.contributor.authorFord, Michael J
dc.contributor.authorDai, Sheng
dc.contributor.authorQiao, Shizhang
dc.contributor.authorShapter, Joseph G
dc.date.accessioned2019-10-09T04:00:17Z
dc.date.available2019-10-09T04:00:17Z
dc.date.issued2018
dc.identifier.issn1433-7851
dc.identifier.doi10.1002/anie.201712280
dc.identifier.urihttp://hdl.handle.net/10072/388163
dc.description.abstractResearch into efficient synthesis, fundamental properties, and potential applications of phosphorene is currently the subject of intense investigation. Herein, solution-processed phosphorene or few-layer black phosphorus (FL-BP) sheets are prepared using a microwave exfoliation method and used in photoelectrochemical cells. Based on experimental and theoretical (DFT) studies, the FL-BP sheets are found to act as catalytically active sites and show excellent electrocatalytic activity for triiodide reduction in dye-sensitized solar cells. Importantly, the device fabricated based on the newly designed cobalt sulfide (CoSx) decorated nitrogen and sulfur co-doped carbon nanotube heteroelectrocatalyst coated with FL-BP (FL-BP@N,S-doped CNTs-CoSx) displayed an impressive photovoltaic efficiency of 8.31 %, outperforming expensive platinum based cells. This work paves the way for using phosphorene-based electrocatalysts for next-generation energy-storage systems.
dc.description.peerreviewedYes
dc.languageEnglish
dc.language.isoeng
dc.publisherWiley Blackwell
dc.relation.ispartofpagefrom2644
dc.relation.ispartofpageto2647
dc.relation.ispartofissue10
dc.relation.ispartofjournalAngewandte Chemie, International Edition
dc.relation.ispartofvolume57
dc.subject.fieldofresearchChemical Sciences
dc.subject.fieldofresearchcode03
dc.subject.keywordsScience & Technology
dc.subject.keywordsPhysical Sciences
dc.subject.keywordsChemistry, Multidisciplinary
dc.subject.keywordsChemistry
dc.subject.keywords2D materials
dc.titleElectrocatalytic Activity of a 2D Phosphorene-Based Heteroelectrocatalyst for Photoelectrochemical Cells
dc.typeJournal article
dc.type.descriptionC1 - Articles
dcterms.bibliographicCitationBatmunkh, M; Shrestha, A; Bat-Erdene, M; Nine, MJ; Shearer, CJ; Gibson, CT; Slattery, AD; Tawfik, SA; Ford, MJ; Dai, S; Qiao, S; Shapter, JG, Electrocatalytic Activity of a 2D Phosphorene-Based Heteroelectrocatalyst for Photoelectrochemical Cells, Angewandte Chemie, International Edition, 2018, 57 (10), pp. 2644-2647
dc.date.updated2019-10-09T03:54:27Z
dc.description.versionAccepted Manuscript (AM)
gro.rights.copyright© 2018 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. This is the peer reviewed version of the following article: Electrocatalytic Activity of a 2D Phosphorene‐Based Heteroelectrocatalyst for Photoelectrochemical Cells, Angewandte Chemie, International Edition, Volume 57, Issue 10, Pages 2644-2647, 2018, which has been published in final form at https://doi.org/10.1002/anie.201712280. This article may be used for non-commercial purposes in accordance with Wiley Terms and Conditions for Self-Archiving (http://olabout.wiley.com/WileyCDA/Section/id-828039.html)
gro.hasfulltextFull Text
gro.griffith.authorBatmunkh, Munkhbayar
gro.griffith.authorBat-Erdene, Munkhjargal


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