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  • Enhanced CO2 electroreduction performance over Cl-modified metal catalysts

    Author(s)
    Fu, Huai Qin
    Zhang, Le
    Zheng, Li Rong
    Liu, Peng Fei
    Zhao, Huijun
    Yang, Hua Gui
    Griffith University Author(s)
    Yang, Huagui
    Zhao, Huijun
    Fu, Huai Qin
    Year published
    2019
    Metadata
    Show full item record
    Abstract
    Ag nanoparticles with surface Cl− modification (Ag–Cl NPs) by in situ electroreduction of AgCl exhibit a high selectivity for CO2-to-CO conversion. The observed C–Cl bond suggests that electrons can be effectively transferred from the Cl− ions to the unoccupied orbital of CO2, and then activate nonpolar CO2 molecules on Cl− sites.Ag nanoparticles with surface Cl− modification (Ag–Cl NPs) by in situ electroreduction of AgCl exhibit a high selectivity for CO2-to-CO conversion. The observed C–Cl bond suggests that electrons can be effectively transferred from the Cl− ions to the unoccupied orbital of CO2, and then activate nonpolar CO2 molecules on Cl− sites.
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    Journal Title
    Journal of Materials Chemistry A
    Volume
    7
    Issue
    20
    DOI
    https://doi.org/10.1039/c9ta02223f
    Subject
    Macromolecular and materials chemistry
    Materials engineering
    Other engineering
    Science & Technology
    Physical Sciences
    Technology
    Chemistry, Physical
    Energy & Fuels
    Publication URI
    http://hdl.handle.net/10072/388379
    Collection
    • Journal articles

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