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dc.contributor.authorAbdelhamid, Muhammad E
dc.contributor.authorRuether, Thomas
dc.contributor.authorVeder, Jean-Pierre
dc.contributor.authorRodopoulos, Theo
dc.contributor.authorBhatt, Anand I
dc.contributor.authorLee, Junqiao
dc.contributor.authorHollenkamp, Anthony F
dc.contributor.authorHorne, Mike D
dc.contributor.authorThuy, Huynh
dc.contributor.authorOng, Andojo
dc.contributor.authorPutman, Kate J
dc.contributor.authorRowe, Genna
dc.contributor.authorde Souza, Paulo
dc.date.accessioned2020-01-24T06:10:24Z
dc.date.available2020-01-24T06:10:24Z
dc.date.issued2019
dc.identifier.issn0013-4651
dc.identifier.doi10.1149/2.0601903jes
dc.identifier.urihttp://hdl.handle.net/10072/390892
dc.description.abstractSolid state microbatteries are highly sought after for emerging microsensor technologies. To overcome the problem of the dwarfing capacity resulting from the miniaturization of the battery, 3D-structured platform consisting of high surface area micropillar-shaped electrodes are used. However, applying a conformal and continuous solid polymer electrolyte films onto the intricate 3D electrodes is a crucial step toward achieving functional microbatteries. In this work, we present our approach for the development of polyethylene oxide (PEO)-acrylate based ion conducting polymer thin films which function as solid polymer electrolyte (SPE) and a separator. The SPEs were electrochemically deposited on the 3D electrodes resulting in ultrathin, continuous, conformal, and pinhole-free polymer films. The electrochemical and Li+ ions transport properties of the SPEs were characterized by EIS measurements and cyclic voltammetry. Furthermore, the homogenous composition of the SPEs at various depths were confirmed by XPS depth profiling techniques.
dc.description.peerreviewedYes
dc.languageEnglish
dc.language.isoeng
dc.publisherElectrochemical Society
dc.relation.ispartofpagefromA5462
dc.relation.ispartofpagetoA5469
dc.relation.ispartofissue3
dc.relation.ispartofjournalJournal of the Electrochemical Society
dc.relation.ispartofvolume166
dc.subject.fieldofresearchMacromolecular and Materials Chemistry
dc.subject.fieldofresearchPhysical Chemistry (incl. Structural)
dc.subject.fieldofresearchMaterials Engineering
dc.subject.fieldofresearchcode0303
dc.subject.fieldofresearchcode0306
dc.subject.fieldofresearchcode0912
dc.subject.keywordsScience & Technology
dc.subject.keywordsPhysical Sciences
dc.subject.keywordsTechnology
dc.subject.keywordsElectrochemistry
dc.subject.keywordsMaterials Science, Coatings & Films
dc.titleElectrochemically Controlled Deposition of Ultrathin Polymer Electrolyte on Complex Microbattery Electrode Architectures
dc.typeJournal article
dc.type.descriptionC1 - Articles
dcterms.bibliographicCitationAbdelhamid, ME; Ruether, T; Veder, J-P; Rodopoulos, T; Bhatt, AI; Lee, J; Hollenkamp, AF; Horne, MD; Thuy, H; Ong, A; Putman, KJ; Rowe, G; de Souza, P, Electrochemically Controlled Deposition of Ultrathin Polymer Electrolyte on Complex Microbattery Electrode Architectures, Journal of the Electrochemical Society, 2019, 166 (3), pp. A5462-A5469
dcterms.licensehttp://creativecommons.org/licenses/by/4.0/
dc.date.updated2020-01-24T05:54:26Z
dc.description.versionVersion of Record (VoR)
gro.rights.copyright© The Author(s) 2019. This is an open access article distributed under the terms of the Creative Commons Attribution 4.0 License, which permits unrestricted reuse of the work in any medium, provided the original work is properly cited.
gro.hasfulltextFull Text
gro.griffith.authorDe Souza Junior, Paulo A.


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