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dc.contributor.authorWu, Shenghao
dc.contributor.authorYang, Huachao
dc.contributor.authorXiong, Guoping
dc.contributor.authorTian, Yikuan
dc.contributor.authorGong, Biyao
dc.contributor.authorLuo, Tengfei
dc.contributor.authorFisher, Timothy S
dc.contributor.authorYan, Jianhua
dc.contributor.authorCen, Kefa
dc.contributor.authorBo, Zheng
dc.contributor.authorOstrikov, Kostya Ken
dc.date.accessioned2020-03-23T00:20:44Z
dc.date.available2020-03-23T00:20:44Z
dc.date.issued2019
dc.identifier.issn1936-0851
dc.identifier.doi10.1021/acsnano.9b05703
dc.identifier.urihttp://hdl.handle.net/10072/392525
dc.description.abstractOil spills remain a worldwide challenge and need emergency “spill-SOS” actions when they occur. Conventional methods suffer from complex processes and high cost. Here, we demonstrate a solar-heating siphon-capillary oil skimmer (S-SOS) that harvests solar energy, gravitational potential energy, and solid surface energy to enable efficient oil spill recovery in a self-pumping manner. The S-SOS is assembled by an inverted U-shape porous architecture combining solar-heating, siphon, and capillary effects, and works without any external power or manual interventions. Importantly, solid surface energy is used by capillary adsorption to enable the self-starting behavior, gravitational potential energy is utilized by siphon transport to drive the oil flow, and solar energy is harvested by solar-thermal conversion to facilitate the transport speed. In the proof-of-concept work, an all-carbon hierarchical architecture (VG/GF) is fabricated by growing vertically oriented graphene nanosheets (VGs) on a monolith of graphite felt (GF) via a plasma-enhanced method to serve as the U-shape architecture. Consequently, an oil-recovery rate of 35.2 L m–2 h–1 is obtained at ambient condition. When exposed to normal solar irradiation, the oil-recovery rate dramatically increases to 123.3 L m–2 h–1. Meanwhile, the solar-thermal energy efficiency is calculated to be 75.3%. Moreover, the S-SOS system presents excellent stability without obvious performance-degradation over 60 h. The outstanding performance is ascribed to the enhanced siphon action, capillary action, photonic absorption, and interfacial heating in the plasma-made graphene nanostructures. Multiple merits make the current S-SOS design and the VG/GF nanostructures promising for efficient oil recovery and transport of energy stored in chemical bonds.
dc.description.peerreviewedYes
dc.languageEnglish
dc.language.isoeng
dc.publisherAmerican Chemical Society
dc.relation.ispartofpagefrom13027
dc.relation.ispartofpageto13036
dc.relation.ispartofissue11
dc.relation.ispartofjournalACS Nano
dc.relation.ispartofvolume13
dc.subject.fieldofresearchNanotechnology
dc.subject.fieldofresearchcode1007
dc.subject.keywordsScience & Technology
dc.subject.keywordsPhysical Sciences
dc.subject.keywordsTechnology
dc.subject.keywordsChemistry, Multidisciplinary
dc.subject.keywordsChemistry, Physical
dc.titleSpill-SOS: Self-Pumping Siphon-Capillary Oil Recovery
dc.typeJournal article
dc.type.descriptionC1 - Articles
dcterms.bibliographicCitationWu, S; Yang, H; Xiong, G; Tian, Y; Gong, B; Luo, T; Fisher, TS; Yan, J; Cen, K; Bo, Z; Ostrikov, KK, Spill-SOS: Self-Pumping Siphon-Capillary Oil Recovery, ACS Nano, 2019, 13 (11), pp. 13027-13036
dc.date.updated2020-03-23T00:18:45Z
gro.hasfulltextNo Full Text
gro.griffith.authorOstrikov, Kostya (Ken)


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