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  • Imaging the time-dependent structure of a molecule as it undergoes dynamics

    Author(s)
    Legare, F
    Lee, KF
    Litvinyuk, IV
    Dooley, PW
    Bandrauk, AD
    Villeneuve, DM
    Corkum, PB
    Griffith University Author(s)
    Litvinyuk, Igor
    Year published
    2005
    Metadata
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    Abstract
    We image the dynamics of diatomic and triatomic molecules with sub-5 fs and sub-A resolution using laser Coulomb explosion imaging with 8 fs pulses. We obtain image information by measuring the vector momenta of all atomic ions produced by explosion of a single molecule. We image vibrating D{sub 2}{sup +} and of dissociating SO{sub 2}{sup 2+} and SO{sub 2}{sup 3+}. Images taken at 0 and 60 fs show that the dissociation of SO{sub 2}{sup 2+} produces an SO{sup +} rotational wave packet.We image the dynamics of diatomic and triatomic molecules with sub-5 fs and sub-A resolution using laser Coulomb explosion imaging with 8 fs pulses. We obtain image information by measuring the vector momenta of all atomic ions produced by explosion of a single molecule. We image vibrating D{sub 2}{sup +} and of dissociating SO{sub 2}{sup 2+} and SO{sub 2}{sup 3+}. Images taken at 0 and 60 fs show that the dissociation of SO{sub 2}{sup 2+} produces an SO{sup +} rotational wave packet.
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    Journal Title
    Physical Review A (Atomic, Molecular and Optical Physics)
    Volume
    72
    Issue
    5
    DOI
    https://doi.org/10.1103/PhysRevA.72.052717
    Subject
    Mathematical sciences
    Physical sciences
    Atomic and molecular physics
    Chemical sciences
    Publication URI
    http://hdl.handle.net/10072/39402
    Collection
    • Journal articles

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