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dc.contributor.authorLiu, L
dc.contributor.authorYang, X
dc.contributor.authorXie, Y
dc.contributor.authorLiu, H
dc.contributor.authorZhou, X
dc.contributor.authorXiao, X
dc.contributor.authorRen, Y
dc.contributor.authorMa, Z
dc.contributor.authorCheng, X
dc.contributor.authorDeng, Y
dc.contributor.authorZhao, D
dc.date.accessioned2020-07-10T04:59:42Z
dc.date.available2020-07-10T04:59:42Z
dc.date.issued2020
dc.identifier.issn0935-9648
dc.identifier.doi10.1002/adma.201906653
dc.identifier.urihttp://hdl.handle.net/10072/395333
dc.description.abstractThe advantages of existing ordered mesoporous materials have not yet been fully realized, due to their limited accessibility of in‐pore surface and long mass‐diffusion length. A general, controllable, and scalable synthesis of a family of two‐dimensional (2D) single‐layer ordered mesoporous materials (SOMMs) with completely exposed mesopore channels, significantly improved mass diffusion, and diverse framework composition is reported here. The SOMMs are synthesized via a surface‐limited cooperative assembly (SLCA) on water‐removable substrates of inorganic salts (e.g., NaCl), combined with vacuum filtration. As a proof of concept, the obtained CeO2‐based SOMMs show superior catalytic performance in CO oxidation with high conversion efficiency, ≈33 times higher than that of conventional bulk mesoporous CeO2. This SLCA is a promising approach for developing next‐generation porous materials for various applications.
dc.description.peerreviewedYes
dc.languageEnglish
dc.language.isoeng
dc.publisherWiley
dc.relation.ispartofpagefrome1906653
dc.relation.ispartofissue10
dc.relation.ispartofjournalAdvanced Materials
dc.relation.ispartofvolume32
dc.subject.fieldofresearchPhysical Sciences
dc.subject.fieldofresearchChemical Sciences
dc.subject.fieldofresearchEngineering
dc.subject.fieldofresearchcode02
dc.subject.fieldofresearchcode03
dc.subject.fieldofresearchcode09
dc.subject.keywordsnanosheets
dc.subject.keywordsordered mesoporous materials
dc.subject.keywordssingle layers
dc.titleA Universal Lab-on-Salt-Particle Approach to 2D Single-Layer Ordered Mesoporous Materials
dc.typeJournal article
dc.type.descriptionC1 - Articles
dcterms.bibliographicCitationLiu, L; Yang, X; Xie, Y; Liu, H; Zhou, X; Xiao, X; Ren, Y; Ma, Z; Cheng, X; Deng, Y; Zhao, D, A Universal Lab-on-Salt-Particle Approach to 2D Single-Layer Ordered Mesoporous Materials, Advanced Materials, 2020, 32 (10), pp. e1906653
dc.date.updated2020-07-10T04:55:33Z
gro.hasfulltextNo Full Text
gro.griffith.authorZhao, Dongyuan


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