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  • Portable wastewater treatment system based on synergistic photocatalytic and persulphate degradation under visible light

    Author(s)
    Zu, M
    Zhang, S
    Liu, C
    Liu, P
    Li, DS
    Xing, C
    Zhang, S
    Griffith University Author(s)
    Liu, Porun
    Zu, Meng
    Zhang, Shanqing
    Xing, Chao
    Year published
    2021
    Metadata
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    Abstract
    Highly efficient, low-cost, and portable wastewater treatment and purification solutions are urgently needed for aqueous pollution removal, especially at remote sites. Synergistic photocatalytic (PC) and persulphate (PS) degradation under visible light offers an exceptional alternative for this purpose. In this work, we coupled a TiO2-based PC system with a PS oxidation system into a portable advanced oxidation device for rapid and deep degradation of organic contaminants in wastewater. Using hydrogenation, we fabricated hydrogenated anatase branched-rutile TiO2 nanorod (H-AB@RTNR) photocatalysts which enable the PC degradation ...
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    Highly efficient, low-cost, and portable wastewater treatment and purification solutions are urgently needed for aqueous pollution removal, especially at remote sites. Synergistic photocatalytic (PC) and persulphate (PS) degradation under visible light offers an exceptional alternative for this purpose. In this work, we coupled a TiO2-based PC system with a PS oxidation system into a portable advanced oxidation device for rapid and deep degradation of organic contaminants in wastewater. Using hydrogenation, we fabricated hydrogenated anatase branched-rutile TiO2 nanorod (H-AB@RTNR) photocatalysts which enable the PC degradation to occur under visible light and improve the utilization of solar energy. We also discovered that the addition of PS resulted in the synergistic degradation of tenacious and persistent organics, dramatically improving the extent and kinetics of the degradation. A degradation rate of 100% and a reaction rate constant of 0.0221 min−1 for degrading 1 L rhodamine B (20 mg L−1) were achieved in 120 min in a specially designed thin-layer cell under visible light irradiation. The superior performance of the synergistic PC and PS degradation system was also demonstrated in the degradation of real industrial wastewater. Both remarkable performances can be attributed to the heterophase junction and oxygen vacancies in the photocatalyst that facilitate the catalytic conversion of PS anions into highly active radicals (·SO4− and ·OH). This work suggests that the as proposed synergistic degradation design is a promising solution for building a portable wastewater treatment system.
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    Journal Title
    Science China Materials
    DOI
    https://doi.org/10.1007/s40843-020-1599-2
    Note
    This publication has been entered in Griffith Research Online as an advanced online version.
    Subject
    Environmental Engineering
    Publication URI
    http://hdl.handle.net/10072/403378
    Collection
    • Journal articles

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