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dc.contributor.authorDou, Yuhai
dc.contributor.authorWang, Yunxiao
dc.contributor.authorTian, Dongliang
dc.contributor.authorXu, Jiantie
dc.contributor.authorZhang, Zhijia
dc.contributor.authorLiu, Qiannan
dc.contributor.authorRuan, Boyang
dc.contributor.authorMa, Jianmin
dc.contributor.authorSun, Ziqi
dc.contributor.authorDou, Shi Xue
dc.date.accessioned2021-06-23T06:07:24Z
dc.date.available2021-06-23T06:07:24Z
dc.date.issued2017
dc.identifier.issn2053-1583en_US
dc.identifier.doi10.1088/2053-1583/4/1/015022en_US
dc.identifier.urihttp://hdl.handle.net/10072/405292
dc.description.abstractCapacitive storage (e.g., double layer capacitance and pseudocapacitance) with Na+ stored mainly at the surface or interface of the active materials rather than inserted into the bulk crystal is an effective approach to achieve high rate capability and long cycle life in sodium-ion batteries (SIBs). Herein, atomically thin Co3O4 nanosheets are successfully synthesized and grown directly on the stainless steel mesh as an anode material for SIBs. This anode delivers a high average capacity of 509.2 mAh g-1 for the initial 20 cycles (excluding the first cycle) at 50 mA g-1, presents excellent rate capability with an average capacity of 427.0 mAh g-1 at 500 mA g-1, and exhibits high cycling stability, which significantly outperforms the electrode prepared from conventional Co3O4 nanostructures, the electrode prepared by conventional casting method, and previously reported Co3O4 electrodes. The superior electrochemical performance is mainly attributable to the atomic thickness of the Co3O4 nanosheets and the direct growth method in electrode processing, which lead to remarkably enhanced surface redox pseudocapacitance and interfacial double layer capacitance. This Na+ capacitive storage mechanism provides a promising strategy for the development of electrode materials with high energy and power densities and ultralong cycle life for SIBs.en_US
dc.description.peerreviewedYesen_US
dc.languageEnglishen_US
dc.publisherIOP Publishing Ltden_US
dc.relation.ispartofpagefrom015022en_US
dc.relation.ispartofissue1en_US
dc.relation.ispartofjournal2D Materialsen_US
dc.relation.ispartofvolume4en_US
dc.subject.fieldofresearchMacromolecular and Materials Chemistryen_US
dc.subject.fieldofresearchMaterials Engineeringen_US
dc.subject.fieldofresearchNanotechnologyen_US
dc.subject.fieldofresearchcode0303en_US
dc.subject.fieldofresearchcode0912en_US
dc.subject.fieldofresearchcode1007en_US
dc.subject.keywordsScience & Technologyen_US
dc.subject.keywordsTechnologyen_US
dc.subject.keywordsMaterials Science, Multidisciplinaryen_US
dc.subject.keywordsMaterials Scienceen_US
dc.subject.keywordsatomically thinen_US
dc.titleAtomically thin Co3O4 nanosheet-coated stainless steel mesh with enhanced capacitive Na+ storage for high-performance sodium-ion batteriesen_US
dc.typeJournal articleen_US
dc.type.descriptionC1 - Articlesen_US
dcterms.bibliographicCitationDou, Y; Wang, Y; Tian, D; Xu, J; Zhang, Z; Liu, Q; Ruan, B; Ma, J; Sun, Z; Dou, SX, Atomically thin Co3O4 nanosheet-coated stainless steel mesh with enhanced capacitive Na+ storage for high-performance sodium-ion batteries, 2D Materials, 2017, 4 (1), pp. 015022en_US
dc.date.updated2021-06-23T05:04:38Z
gro.hasfulltextNo Full Text
gro.griffith.authorDou, Yuhai


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