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dc.contributor.authorLiu, S
dc.contributor.authorZhang, X
dc.contributor.authorWang, G
dc.contributor.authorZhang, Y
dc.contributor.authorZhang, H
dc.date.accessioned2021-06-25T04:50:53Z
dc.date.available2021-06-25T04:50:53Z
dc.date.issued2017
dc.identifier.issn1944-8244
dc.identifier.doi10.1021/acsami.7b11101
dc.identifier.urihttp://hdl.handle.net/10072/405376
dc.description.abstractDeveloping bifunctional oxygen electrocatalysts with superior catalytic activities of oxygen reduction reaction (ORR) and oxygen revolution reaction (OER) is crucial to their practical energy storage and conversion applications. In this work, we report the fabrication of Co/CoxSy@S,N-codoped porous carbon structures with various morphologies, specific surface areas, and pore structures, derived from controllably grown Co-based metal–organic frameworks with S- and N-containing organic ligands (thiophene-2,5-dicarboxylate, Tdc; and 4,4′-bipyridine, bpy) utilizing solvent effect (e.g., water and methanol) under room temperature and hydrothermal conditions. The results demonstrate that Co/CoxSy@S,N-codoped carbon fibers fabricated at a pyrolytic temperature of 800 °C (Co/CoxSy@SNCF-800) from Co-MOFs fibers fabricated in methanol under hydrothermal conditions as electrocatalysts exhibit superior bifunctional ORR and OER activities in alkaline media, endowing them as air cathodic catalysts in rechargeable zinc–air batteries with high power density and good durability.
dc.description.peerreviewedYes
dc.languageeng
dc.publisherAmerican Chemical Society
dc.relation.ispartofpagefrom34269
dc.relation.ispartofpageto34278
dc.relation.ispartofissue39
dc.relation.ispartofjournalACS Applied Materials & Interfaces
dc.relation.ispartofvolume9
dc.subject.fieldofresearchChemical sciences
dc.subject.fieldofresearchEngineering
dc.subject.fieldofresearchcode34
dc.subject.fieldofresearchcode40
dc.subject.keywordsS, N dual organic ligands
dc.subject.keywordsZn−air battery
dc.subject.keywords[Co(Tdc)(bpy)]n
dc.subject.keywordsbifunctional oxygen electrocatalysts
dc.subject.keywordssolvent effect
dc.titleHigh-Efficiency Co/CoxSy@S,N-Codoped Porous Carbon Electrocatalysts Fabricated from Controllably Grown Sulfur- and Nitrogen-Including Cobalt-Based MOFs for Rechargeable Zinc–Air Batteries
dc.typeJournal article
dc.type.descriptionC1 - Articles
dcterms.bibliographicCitationLiu, S; Zhang, X; Wang, G; Zhang, Y; Zhang, H, High-Efficiency Co/CoxSy@S,N-Codoped Porous Carbon Electrocatalysts Fabricated from Controllably Grown Sulfur- and Nitrogen-Including Cobalt-Based MOFs for Rechargeable Zinc–Air Batteries, ACS Applied Materials & Interfaces, 2017, 9 (39), pp. 34269-34278
dc.date.updated2021-06-25T04:47:10Z
gro.hasfulltextNo Full Text
gro.griffith.authorZhang, Haimin


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