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dc.contributor.authorLin, ZQ
dc.contributor.authorQiao, HW
dc.contributor.authorZhou, ZR
dc.contributor.authorHou, Y
dc.contributor.authorLi, X
dc.contributor.authorYang, HG
dc.contributor.authorYang, S
dc.date.accessioned2021-07-15T22:58:13Z
dc.date.available2021-07-15T22:58:13Z
dc.date.issued2020
dc.identifier.issn2050-7488
dc.identifier.doi10.1039/d0ta05118g
dc.identifier.urihttp://hdl.handle.net/10072/406016
dc.description.abstractCesium lead halide perovskites are promising alternatives as light-absorbing materials for achieving perovskite solar cells with excellent thermal stability, but their inferior power conversion efficiency (PCE) and ambient instability are impeding their application. In this work, we show that liquid water can assist the formation of CsPbI2Br perovskites under the synergetic adsorption of H2O and dimethylsulfoxide (DMSO), which enabled uniform, [100] oriented CsPbI2Br films with a grain size up to 4.4 μm. It was found that a suitable amount of H2O helps desorb the DMSO molecules, and thus favours the formation of a cubic perovskite phase from DMSO complexed intermediates. Perovskite solar cells based on our strategy delivered an optimized PCE of 16.47% with a high open-voltage of 1.33 V, as well as good device stability against humidity, light and heat.
dc.description.peerreviewedYes
dc.languageen
dc.publisherRoyal Society of Chemistry (RSC)
dc.relation.ispartofpagefrom17670
dc.relation.ispartofpageto17674
dc.relation.ispartofissue34
dc.relation.ispartofjournalJournal of Materials Chemistry A
dc.relation.ispartofvolume8
dc.subject.fieldofresearchMacromolecular and materials chemistry
dc.subject.fieldofresearchMaterials engineering
dc.subject.fieldofresearchOther engineering
dc.subject.fieldofresearchcode3403
dc.subject.fieldofresearchcode4016
dc.subject.fieldofresearchcode4099
dc.titleWater assisted formation of highly oriented CsPbI2Br perovskite films with the solar cell efficiency exceeding 16%
dc.typeJournal article
dc.type.descriptionC1 - Articles
dcterms.bibliographicCitationLin, ZQ; Qiao, HW; Zhou, ZR; Hou, Y; Li, X; Yang, HG; Yang, S, Water assisted formation of highly oriented CsPbI2Br perovskite films with the solar cell efficiency exceeding 16%, Journal of Materials Chemistry A, 2020, 8 (34), pp. 17670-17674
dc.date.updated2021-07-15T11:27:04Z
gro.hasfulltextNo Full Text
gro.griffith.authorYang, Huagui


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