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dc.contributor.authorArandiyan, Hamidreza
dc.contributor.authorMofarah, Sajjad S
dc.contributor.authorSorrell, Charles C
dc.contributor.authorDoustkhah, Esmail
dc.contributor.authorSajjadi, Baharak
dc.contributor.authorHao, Derek
dc.contributor.authorWang, Yuan
dc.contributor.authorSun, Hongyu
dc.contributor.authorNi, Bing-Jie
dc.contributor.authorRezaei, Mehran
dc.contributor.authorShao, Zongping
dc.contributor.authorMaschmeyer, Thomas
dc.date.accessioned2021-11-18T01:02:53Z
dc.date.available2021-11-18T01:02:53Z
dc.date.issued2021
dc.identifier.issn0306-0012en_US
dc.identifier.doi10.1039/d0cs00639den_US
dc.identifier.urihttp://hdl.handle.net/10072/410199
dc.description.abstractOxide perovskites have emerged as an important class of materials with important applications in many technological areas, particularly thermocatalysis, electrocatalysis, photocatalysis, and energy storage. However, their implementation faces numerous challenges that are familiar to the chemist and materials scientist. The present work surveys the state-of-the-art by integrating these two viewpoints, focusing on the critical role that defect engineering plays in the design, fabrication, modification, and application of these materials. An extensive review of experimental and simulation studies of the synthesis and performance of oxide perovskites and devices containing these materials is coupled with exposition of the fundamental and applied aspects of defect equilibria. The aim of this approach is to elucidate how these issues can be integrated in order to shed light on the interpretation of the data and what trajectories are suggested by them. This critical examination has revealed a number of areas in which the review can provide a greater understanding. These include considerations of (1) the nature and formation of solid solutions, (2) site filling and stoichiometry, (3) the rationale for the design of defective oxide perovskites, and (4) the complex mechanisms of charge compensation and charge transfer. The review concludes with some proposed strategies to address the challenges in the future development of oxide perovskites and their applications.en_US
dc.description.peerreviewedYesen_US
dc.languageEnglishen_US
dc.publisherRoyal Society of Chemistryen_US
dc.relation.ispartofpagefrom10116en_US
dc.relation.ispartofpageto10211en_US
dc.relation.ispartofissue18en_US
dc.relation.ispartofjournalChemical Society Reviewsen_US
dc.relation.ispartofvolume50en_US
dc.subject.fieldofresearchNanomaterialsen_US
dc.subject.fieldofresearchInorganic chemistryen_US
dc.subject.fieldofresearchEngineeringen_US
dc.subject.fieldofresearchcode401807en_US
dc.subject.fieldofresearchcode3402en_US
dc.subject.fieldofresearchcode40en_US
dc.subject.keywordsScience & Technologyen_US
dc.subject.keywordsPhysical Sciencesen_US
dc.subject.keywordsChemistry, Multidisciplinaryen_US
dc.subject.keywordsChemistryen_US
dc.subject.keywordsOXYGEN REDUCTION REACTIONen_US
dc.titleDefect engineering of oxide perovskites for catalysis and energy storage: synthesis of chemistry and materials scienceen_US
dc.typeJournal articleen_US
dc.type.descriptionC1 - Articlesen_US
dcterms.bibliographicCitationArandiyan, H; Mofarah, SS; Sorrell, CC; Doustkhah, E; Sajjadi, B; Hao, D; Wang, Y; Sun, H; Ni, B-J; Rezaei, M; Shao, Z; Maschmeyer, T, Defect engineering of oxide perovskites for catalysis and energy storage: synthesis of chemistry and materials science, Chemical Society Reviews, 2021, 50 (18), pp. 10116-10211en_US
dc.date.updated2021-11-17T01:39:01Z
gro.hasfulltextNo Full Text
gro.griffith.authorHao, Derek


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