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  • Controllable design of nanoworm-like nickel sulfides for efficient electrochemical water splitting in alkaline media

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    Hao522077-Accepted.pdf (549.1Kb)
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    Accepted Manuscript (AM)
    Author(s)
    Chen, Z
    Ibrahim, I
    Hao, D
    Liu, X
    Wu, L
    Wei, W
    Su, D
    Ni, B-J
    Griffith University Author(s)
    Hao, Derek
    Year published
    2020
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    Abstract
    Developing cost-effective electrocatalysts for electrochemical water splitting (EWS) is appealing and challenging for sustainable water electrolysis. Currently, nickel sulfides are considered as promising candidates for EWS due to their low cost and high catalytic activity. However, the facile design of nickel sulfides with high catalytic performance is still highly demanded. In this study, we have developed a one-step solvothermal strategy to construct nickel sulfides as efficient water splitting catalysts. By taking advantage of the small size, abundant active sites, large electrochemical surface area, and good conductivity, ...
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    Developing cost-effective electrocatalysts for electrochemical water splitting (EWS) is appealing and challenging for sustainable water electrolysis. Currently, nickel sulfides are considered as promising candidates for EWS due to their low cost and high catalytic activity. However, the facile design of nickel sulfides with high catalytic performance is still highly demanded. In this study, we have developed a one-step solvothermal strategy to construct nickel sulfides as efficient water splitting catalysts. By taking advantage of the small size, abundant active sites, large electrochemical surface area, and good conductivity, the nanoworm-like nickel sulfides (NiS-NW/Ni foam [NF]) exhibit better oxygen evolution reaction performance (a low overpotential of 279 mV to achieve 100 mA cm−2, Tafel slope of 38.44 mV dce−1) than the nanoplate-like analogs, as well as most of reported nickel sulfide–based electrocatalysts. In addition, the NiS-NW/NF directly used as bifunctional electrodes for overall water splitting requires a low voltage of 1.563 V to attain a current density of 10 mA cm−2 with good long-term durability. This work provides a facile strategy for the design of efficient nickel sulfide-based electrocatalysts for energy conversion applications.
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    Journal Title
    Materials Today Energy
    Volume
    18
    DOI
    https://doi.org/10.1016/j.mtener.2020.100573
    Copyright Statement
    © 2020 Elsevier. Licensed under the Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 International Licence (http://creativecommons.org/licenses/by-nc-nd/4.0/) which permits unrestricted, non-commercial use, distribution and reproduction in any medium, providing that the work is properly cited.
    Subject
    Electrochemical energy storage and conversion
    Science & Technology
    Physical Sciences
    Chemistry, Physical
    Energy & Fuels
    Publication URI
    http://hdl.handle.net/10072/412047
    Collection
    • Journal articles

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