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  • The Chemistry of the Polycyclic Polyprenylated Acylphloroglucinols

    Author(s)
    Richard, Jean-Alexandre
    H. Pouwer, Rebecca
    Y.-K. Chen, David
    Griffith University Author(s)
    Pouwer, Rebecca
    Year published
    2012
    Metadata
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    Abstract
    With their fascinating biological profiles and stunningly complex molecular architectures, the polycyclic polyprenylated acylphloroglucinols (PPAPs) have long provided a fertile playing field for synthetic organic chemists. In particular, the recent advent of innovative synthetic methods and strategies together with C[BOND]C bond-forming reactions and asymmetric catalysis have revitalized this field tremendously. Consequently, PPAP targets which once seemed beyond reach have now been synthesized. This Review aims to highlight the recent achievements in the total synthesis of PPAPs, as well as notable methods developed for ...
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    With their fascinating biological profiles and stunningly complex molecular architectures, the polycyclic polyprenylated acylphloroglucinols (PPAPs) have long provided a fertile playing field for synthetic organic chemists. In particular, the recent advent of innovative synthetic methods and strategies together with C[BOND]C bond-forming reactions and asymmetric catalysis have revitalized this field tremendously. Consequently, PPAP targets which once seemed beyond reach have now been synthesized. This Review aims to highlight the recent achievements in the total synthesis of PPAPs, as well as notable methods developed for the construction of the bicyclo[3.3.1] core of these chemically and biologically intriguing molecules.
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    Journal Title
    Angewandte Chemie – International Edition
    Volume
    51
    Issue
    19
    DOI
    https://doi.org/10.1002/anie.201103873
    Subject
    Organic Chemical Synthesis
    Chemical Sciences
    Publication URI
    http://hdl.handle.net/10072/50840
    Collection
    • Journal articles

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