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  • Novel lithium-loaded porous aromatic framework for efficient CO2 and H2 uptake

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    Author(s)
    Ma, Heping
    Ren, Hao
    Zou, Xiaoqin
    Sun, Fuxing
    Yan, Zhuojun
    Cai, Kun
    Wang, Dayang
    Zhu, Guangshan
    Griffith University Author(s)
    Zhu, Guangshan
    Year published
    2013
    Metadata
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    Abstract
    Novel porous aromatic frameworks, PAF-18-OH and its lithiated derivative PAF-18-OLi, have been successfully synthesized. In particular, PAF-18-OLi displays significant enhancement of H2 and CO2 adsorption capacity, especially for CO2 uptake (14.4 wt%). More valuably, the stable PAF-18-OLi material exhibits high CO2/N2 selectivity, as high as 129 in the case of CO2 capture from simulated post-combustion flue gas mixtures (85% N2 and 15% CO2). Furthermore, the PAF-18-OLi has shown improved H2 storage capacity after lithiation.Novel porous aromatic frameworks, PAF-18-OH and its lithiated derivative PAF-18-OLi, have been successfully synthesized. In particular, PAF-18-OLi displays significant enhancement of H2 and CO2 adsorption capacity, especially for CO2 uptake (14.4 wt%). More valuably, the stable PAF-18-OLi material exhibits high CO2/N2 selectivity, as high as 129 in the case of CO2 capture from simulated post-combustion flue gas mixtures (85% N2 and 15% CO2). Furthermore, the PAF-18-OLi has shown improved H2 storage capacity after lithiation.
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    Journal Title
    Journal of Materials Chemistry A
    Volume
    1
    Issue
    3
    DOI
    https://doi.org/10.1039/c2ta00616b
    Copyright Statement
    © 2013 Royal Society of Chemistry. This is the author-manuscript version of this paper. Reproduced in accordance with the copyright policy of the publisher. Please refer to the journal website for access to the definitive, published version.
    Subject
    Inorganic chemistry not elsewhere classified
    Macromolecular and materials chemistry
    Materials engineering
    Publication URI
    http://hdl.handle.net/10072/54322
    Collection
    • Journal articles

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