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  • Core–Shell Palladium Nanoparticle@Metal–Organic Frameworks as Multifunctional Catalysts for Cascade Reactions

    Author(s)
    Zhao, Meiting
    Deng, Ke
    He, Liangcan
    Liu, Yong
    Li, Guodong
    Zhao, Huijun
    Tang, Zhiyong
    Griffith University Author(s)
    Zhao, Huijun
    Year published
    2014
    Metadata
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    Abstract
    Uniform core-shell Pd@IRMOF-3 nanostructures, where single Pd nanoparticle core is surrounded by amino-functionalized IRMOF-3 shell, are prepared by a facile mixed solvothermal method. When used as multifunctional catalysts, the Pd@IRMOF-3 nanocomposites exhibit high activity, enhanced selectivity, and excellent stability in the cascade reaction. Both experimental evidence and theoretical calculations reveal that the high catalytic performance of Pd@IRMOF-3 nanocomposites originates from their unique core-shell structures.Uniform core-shell Pd@IRMOF-3 nanostructures, where single Pd nanoparticle core is surrounded by amino-functionalized IRMOF-3 shell, are prepared by a facile mixed solvothermal method. When used as multifunctional catalysts, the Pd@IRMOF-3 nanocomposites exhibit high activity, enhanced selectivity, and excellent stability in the cascade reaction. Both experimental evidence and theoretical calculations reveal that the high catalytic performance of Pd@IRMOF-3 nanocomposites originates from their unique core-shell structures.
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    Journal Title
    Journal of the American Chemical Society
    Volume
    136
    Issue
    5
    DOI
    https://doi.org/10.1021/ja411468e
    Copyright Statement
    Self-archiving of the author-manuscript version is not yet supported by this journal. Please refer to the journal link for access to the definitive, published version or contact the authors for more information.
    Subject
    Chemical sciences
    Inorganic chemistry not elsewhere classified
    Publication URI
    http://hdl.handle.net/10072/66824
    Collection
    • Journal articles

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