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dc.contributor.authorWang, Xianyu
dc.contributor.authorThai, Phong K
dc.contributor.authorLi, Yan
dc.contributor.authorLi, Qingbo
dc.contributor.authorWainwright, David
dc.contributor.authorHawker, Darryl W
dc.contributor.authorMueller, Jochen F
dc.date.accessioned2018-09-05T05:20:51Z
dc.date.available2018-09-05T05:20:51Z
dc.date.issued2016
dc.identifier.issn0269-7491
dc.identifier.doi10.1016/j.envpol.2016.02.020
dc.identifier.urihttp://hdl.handle.net/10072/99934
dc.description.abstractOver recent decades, efforts have been made to reduce human exposure to atmospheric pollutants including polycyclic aromatic hydrocarbons (PAHs) and polychlorinated biphenyls (PCBs) through emission control and abatement. Along with the potential changes in their concentrations resulting from these efforts, profiles of emission sources may have also changed over such extended timeframes. However relevant data are quite limited in the Southern Hemisphere. We revisited two sampling sites in an Australian city, where the concentration data in 1994/5 for atmospheric PAHs and PCBs were available. Monthly air samples from July 2013 to June 2014 at the two sites were collected and analysed for these compounds, using similar protocols to the original study. A prominent seasonal pattern was observed for PAHs with elevated concentrations in cooler months whereas PCB levels showed little seasonal variation. Compared to two decades ago, atmospheric concentrations of ∑13 PAHs (gaseous + particle-associated) in this city have decreased by approximately one order of magnitude and the apparent halving time () was estimated as 6.2 ± 0.56 years. ∑6iPCBs concentrations (median value; gaseous + particle-associated) have decreased by 80% with an estimated of 11 ± 2.9 years. These trends and values are similar to those reported for comparable sites in the Northern Hemisphere. To characterise emission source profiles, samples were also collected from a bushfire event and within a vehicular tunnel. Emissions from bushfires are suggested to be an important contributor to the current atmospheric concentrations of PAHs in this city. This contribution is more important in cooler months, i.e. June, July and August, and its importance may have increased over the last two decades.
dc.description.peerreviewedYes
dc.languageEnglish
dc.language.isoeng
dc.publisherElsevier
dc.relation.ispartofpagefrom223
dc.relation.ispartofpageto231
dc.relation.ispartofjournalEnvironmental Pollution
dc.relation.ispartofvolume213
dc.subject.fieldofresearchAtmospheric sciences not elsewhere classified
dc.subject.fieldofresearchcode370199
dc.titleChanges in atmospheric concentrations of polycyclic aromatic hydrocarbons and polychlorinated biphenyls between the 1990s and 2010s in an Australian city and the role of bushfires as a source
dc.typeJournal article
dc.type.descriptionC1 - Articles
dc.type.codeC - Journal Articles
gro.hasfulltextNo Full Text
gro.griffith.authorHawker, Darryl W.


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