Influence of an atomic resonance on the coherent control of the photoionization process

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Gryzlova, EV
Carpeggiani, P
Popova, MM
Kiselev, MD
Douguet, N
Reduzzi, M
Negro, M
Comby, A
Ahmadi, H
Wanie, V
Castrovilli, MC
Fischer, A
Eng-Johnsson, P
Meyer, M
Bartschat, K
et al.
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2022
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Abstract

In coherent control schemes, pathways connecting an initial and a final state can be independently controlled by manipulating the complex amplitudes of their transition matrix elements. For paths characterized by the absorption of multiple photons, these quantities depend on the magnitude and phase between the intermediate steps, and are expected to be strongly affected by the presence of resonances. We investigate the coherent control of the photoemission process in neon using a phase-controlled two-color extreme ultraviolet pulse with frequency in proximity of an excited energy state. Using helium as a reference, we show that the presence of such a resonance in neon modifies the amplitude and phase of the asymmetric emission of photoelectrons. Theoretical simulations based on perturbation theory are in fair agreement with the experimental observations.

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Physical Review Research

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4

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3

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© The Authors 2022. Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI.

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Atomic, molecular and optical physics

Calculus of variations, mathematical aspects of systems theory and control theory

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Gryzlova, EV; Carpeggiani, P; Popova, MM; Kiselev, MD; Douguet, N; Reduzzi, M; Negro, M; Comby, A; Ahmadi, H; Wanie, V; Castrovilli, MC; Fischer, A; Eng-Johnsson, P; Meyer, M; Bartschat, K; et al., Influence of an atomic resonance on the coherent control of the photoionization process, Physical Review Research, 2022, 4 (3), pp. 033231

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