Temporal asymmetry of fluctuations in nonequilibrium steady states: Links with correlation functions and nonlinear response
File version
Author(s)
Bernhardt, Debra
Rondoni, Lamberto
Griffith University Author(s)
Primary Supervisor
Other Supervisors
Editor(s)
Date
Size
1182828 bytes
File type(s)
application/pdf
Location
License
Abstract
The presence of temporal asymmetries in fluctuation paths of nonequilibrium systems has recently been confirmed numerically in nonequilibrium molecular dynamics simulations of particular deterministic systems. Here we show that this is a common feature of homogeneously driven and thermostatted, reversible, deterministic, chaotic, nonequilibrium systems of interacting particles. This is done by expressing fluctuation paths as correlation functions. The theoretical arguments look rather general, and we expect them to easily extend to other forms of driving and thermostats. The emergence of asymmetry is also justified using the transient time correlation function expression of nonlinear response theory. Numerical simulations are used to verify our arguments.
Journal Title
The Journal of Chemical Physics
Conference Title
Book Title
Edition
Volume
128
Issue
Thesis Type
Degree Program
School
Publisher link
Patent number
Funder(s)
Grant identifier(s)
Rights Statement
Rights Statement
© 2008 American Institute of Physics. This article may be downloaded for personal use only. Any other use requires prior permission of the author and the American Institute of Physics. The following article may be found at http://dx.doi.org/10.1063/1.2894471
Item Access Status
Note
Access the data
Related item(s)
Subject
Physical Sciences
Chemical Sciences
Engineering