High-order harmonic generation in helium: A comparison study

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Bondy, AT
Saha, S
Del Valle, JC
Harth, A
Douguet, N
Hamilton, KR
Bartschat, K
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2024
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Abstract

We report a detailed study of high-order harmonic generation (HHG) in helium. When comparing predictions from a single-active-electron model with those from all-electron simulations, such as the attomesa code and 𝑅-matrix-with-time-dependence method, which can include different numbers of states in the close-coupling expansion, it seems imperative to generate absolute numbers for the HHG spectrum in a well-defined framework. While qualitative agreement in the overall frequency dependence of the spectrum, including the cutoff frequency predicted by a semiclassical model, can be achieved by many models in arbitrary units, only absolute numbers can be used for benchmark comparisons between different approaches.

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Physical Review A

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109

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4

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Bondy, AT; Saha, S; Del Valle, JC; Harth, A; Douguet, N; Hamilton, KR; Bartschat, K, High-order harmonic generation in helium: A comparison study, Physical Review A, 2024, 109 (4), pp. 043113

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