Spatially-resolved rotational microrheology with an optically-trapped sphere

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Bennett, James S
Gibson, Lachlan J
Kelly, Rory M
Brousse, Emmanuel
Baudisch, Bastian
Preece, Daryl
Nieminen, Timo A
Nicholson, Timothy
Heckenberg, Norman R
Rubinsztein-Dunlop, Halina
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2013
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Abstract

We have developed a microrheometer, based on optical tweezers, in which hydrodynamic coupling between the probe and fluid boundaries is dramatically reduced relative to existing microrheometers. Rotational Brownian motion of a birefringent microsphere within an angular optical trap is observed by measuring the polarisation shifts of transmitted light. Data gathered in this manner, in the strongly viscoelastic fluid Celluvisc, quantitatively agree with the results of conventional (bulk) rheometry. Our technique will significantly reduce the smallest sample volumes which may be reliably probed, further extending the study of rare, difficult to obtain or highly nonhomogeneous fluids.

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Scientific Reports

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3

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1

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© The Authors 2013. This work is licensed under a Creative Commons Attribution-NonCommercial-NoDerivs 3.0 Unported License. To view a copy of this license, visit http://creativecommons.org/licenses/by-nc-nd/3.0/

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Science & Technology

Multidisciplinary Sciences

Science & Technology - Other Topics

DIFFUSING-WAVE SPECTROSCOPY

TWEEZERS

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Bennett, JS; Gibson, LJ; Kelly, RM; Brousse, E; Baudisch, B; Preece, D; Nieminen, TA; Nicholson, T; Heckenberg, NR; Rubinsztein-Dunlop, H, Spatially-resolved rotational microrheology with an optically-trapped sphere, SCIENTIFIC REPORTS, 2013, 3 (1), pp. 1759

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