Phonon dephasing and spectral diffusion of quantum emitters in hexagonal boron nitride

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White, Simon
Stewart, Connor
Solntsev, Alexander S
Li, Chi
Toth, Milos
Kianinia, Mehran
Aharonovich, Igor
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2021
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Quantum emitters in hexagonal boron nitride (hBN) are emerging as bright and robust sources of single photons for applications in quantum optics. In this work we present detailed studies on the limiting factors to achieve Fourier transform limited spectral lines. Specifically, we study phonon dephasing and spectral diffusion of quantum emitters in hBN via resonant excitation spectroscopy at cryogenic temperatures. We show that the linewidths of hBN quantum emitters are phonon broadened, even at 5 K, with typical values of the order of ∼1GHz. While spectral diffusion dominates at increasing pump powers, it can be minimized by working well below saturation excitation power. Our results are important for future utilization of quantum emitters in hBN for quantum interference experiments.

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Optica

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8

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9

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© 2021 Optical Society of America under the terms of the OSA Open Access Publishing Agreement. Users are allowed to read, download, copy, distribute, print, search, or link to the full text of the article, or use them for any other lawful purpose, without asking prior permission from the publisher or the Author(s). https://opg.optica.org/library/license_v1.cfm#VOR-OA

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White, S; Stewart, C; Solntsev, AS; Li, C; Toth, M; Kianinia, M; Aharonovich, I, Phonon dephasing and spectral diffusion of quantum emitters in hexagonal boron nitride, Optica, 2021, 8 (9), pp. 1153-1158

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